• 关键词：福岛  核泄漏  ¹³¹I-¹³⁷Cs-²¹⁰Pb-⁷Be  气溶胶传输  贵阳

• 基金项目：国家自然科学基金(No.40873086,40773071, 40830102)

• 万恩源
• 中国科学院地球化学研究所 环境地球化学国家重点实验室,贵阳 550002

• 郑向东
• 中国气象科学研究院,中国气象局大气化学开放实验室,北京 100081

• 万国江
• 中国科学院地球化学研究所 环境地球化学国家重点实验室,贵阳 550002

• 王长生
• 中国科学院地球化学研究所 环境地球化学国家重点实验室,贵阳 550002

• 摘要：2011年3月11日,日本本州9.0级地震引发了福岛核电站核泄漏,以及由此引起的¹³¹I和¹³⁷Cs在全球大气环流传输已引起了重视.理论上也对这种输送路径进行了研究.本文报道2011年3月17日—4月28日在贵阳观风山对气溶胶中天然核素(²¹⁰Pb、⁷Be)和人为核素(¹³¹I、¹³⁷Cs)近地面空气浓度逐周采样的系统对比观测,并结合该时段贵阳离地面500 m高度逐周315 h的气团后向轨迹分析.结果表明:福岛核泄漏污染物通过两条显著的途径输送到贵阳地区.第一条是首波核污染通过全球大气环流传输,由西向东,几乎环绕地球一周,历经约10 d至两周,最终在3月24日—31日从我国的西北地区入侵抵至贵阳;第二条途径则是福岛地区上空的核污染气团受东北天气系统的挤压南移并在低纬度地区再次先后受到东北和东南气流的影响,于4月7日—14日抵达贵阳.核污染的第一条输送路径是全球尺度,第二条是东亚区域尺度.

• Abstract：The 9.0 Ritcher scale earthquake happened on March 11^th, 2011 in the Honshu Island, Japan had caused the radioactivity leakage from the Fukushima Nuclear Power Plant. The leaked artificial nuclides, ¹³¹I and ¹³⁷Cs, and their transport processes in the global atmosphere had drawn great public attention. In this paper, the concentrations of radioactive isotopes ⁷Be, ²¹⁰Pb, ¹³¹I and ¹³⁷Cs at the surface level in weekly aerosol samples obtained at the Guanfenshan Moutain, Guiyang, China from March 17^th to April 28^th, 2011 were reported. The variations of the nuclide concentrations associated with their transport paths were analyzed with 315 h-backward trajectories initialized at 500m from the surface level at Guiyang. The results revealed that there were two evident transport paths for ¹³¹I and ¹³⁷Cs from Fukushima to Guiyang. The first path, along with which radioactive pollution tracers reached Guiyang faster, was from the north-western China. These tracers transported eastward and took 10 days to two weeks to arrive the north-western China before they were detected on March 24^th—31^st in Guiyang. The second path extended south-eastward by the north-east Asian synoptic system at the beginning, then transported south-westward and north-westward before their arrivals on April 7^th -14^th in Guiyang. The first transport path of radioactive pollution tracer from the Fukushima Nuclear Power Plant to Guiyang was in the global scale while the second was in the East Asian regional scale.

• Key words：fukushima  nuclear leakiness  ¹³¹I-¹³⁷Cs-²¹⁰Pb-⁷Be  aerosol transport  Guiyang

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